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A quantum mechanical model of electron field emission from two dimensional materials. Application to graphene

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  • معلومة اضافية
    • Contributors:
      Théorie (LCAR); Laboratoire Collisions Agrégats Réactivité (LCAR); Institut de Recherche sur les Systèmes Atomiques et Moléculaires Complexes (IRSAMC); Institut National des Sciences Appliquées - Toulouse (INSA Toulouse); Institut National des Sciences Appliquées (INSA)-Institut National des Sciences Appliquées (INSA)-Centre National de la Recherche Scientifique (CNRS)-Université Toulouse III - Paul Sabatier (UT3); Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées-Institut National des Sciences Appliquées - Toulouse (INSA Toulouse); Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées-Institut de Recherche sur les Systèmes Atomiques et Moléculaires Complexes (IRSAMC); Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées
    • بيانات النشر:
      HAL CCSD
      American Institute of Physics
    • الموضوع:
      2021
    • Collection:
      Archive ouverte HAL (Hyper Article en Ligne, CCSD - Centre pour la Communication Scientifique Directe)
    • نبذة مختصرة :
      International audience ; We implement a new time-independent perturbative quantum method to study quantitatively electron field emission from two dimensional materials and in particular from graphene. The Bardeen transfer Hamiltonian formalism is coupled to a detailed description of the electronic structure of the material. This calculation method is first validated on the standard Fowler-Nordheim (FN) model of a 3 dimensional (3D) free electron gas. Then, it is used to study emission from a 2 dimensional (2D) free electron gas and from graphene represented by a tight-binding model. In the case of graphene, we show that a full electronic band model of the material is necessary to obtain reasonable results because emission is not restricted to the vicinity of the Fermi level near the Dirac points. The graphene emitted current density follows a modified FN law with respect to the applied field, with a prefactor exponent for the field n ≈ 1.5 intermediate between the one for the cases of 2D (n = 0) and 3D (n = 2) free electron gases. However, the emitted current level is low because the kinetic energy of the electrons corresponds to a motion parallel to the emitting surface which is not efficient in promoting emission. Our study gives a firm ground to the idea that emission from graphene results almost exclusively from defects.
    • Relation:
      hal-03196317; https://hal.archives-ouvertes.fr/hal-03196317; https://hal.archives-ouvertes.fr/hal-03196317/document; https://hal.archives-ouvertes.fr/hal-03196317/file/JAP21-AR-00906.pdf
    • الرقم المعرف:
      10.1063/5.0047771
    • Rights:
      info:eu-repo/semantics/OpenAccess
    • الرقم المعرف:
      edsbas.61999274