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Single-shot X-ray absorption spectroscopy at X-ray free electron lasers

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  • معلومة اضافية
    • Contributors:
      Institut de minéralogie, de physique des matériaux et de cosmochimie (IMPMC); Muséum national d'Histoire naturelle (MNHN)-Institut de recherche pour le développement IRD : UR206-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS); Lawrence Livermore National Laboratory (LLNL); Institut de Physique de Rennes (IPR); Université de Rennes (UR)-Centre National de la Recherche Scientifique (CNRS); SLAC National Accelerator Laboratory (SLAC); Stanford University; Paul Scherrer Institute (PSI); This work was supported by the French Agence Nationale de la Recherche with the ANR IRONFEL ANR-12-PDOC-0011. This project has also received funding from the European Research Council (ERC) under the European Union Horizon 2020 research and innovation program (grant agreement No. 670787 D PLANETDIVE). AK is currently working under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344.; ANR-12-PDOC-0011,IronFEL,Le fer et ses alliages sous conditions extrèmes et sondés par diagnostiques X sur les installations FEL et lasers intenses(2012); European Project: 670787,H2020,ERC-2014-ADG,PLANETDIVE(2016)
    • بيانات النشر:
      HAL CCSD
      Nature Publishing Group
    • الموضوع:
      2023
    • Collection:
      Université de Rennes 1: Publications scientifiques (HAL)
    • نبذة مختصرة :
      International audience ; X-ray Absorption Spectroscopy (XAS) is a widely used diagnostic method for studying electronic and structural properties of matter. At first glance, the relatively narrow bandwidth highly fluctuating spectral structure Free Electron Lasers (XFEL) sources seem to require accumulation over many shots achieve high data quality. To date best approach implementing XAS at XFEL facilities has been using monochromators scan photon energy across desired range. While this possible easily reproducible samples such as liquids, it incompatible with important systems. Here, we demonstrate collection single-shot spectra 10s eV an source, error bars only few percent. We additionally show how extend technique wider ranges towards Extended Fine Structure measurements, by concatenating tens measurements. Our results pave way future studies XFELs, in particular those femtosecond regime. This advance envisioned be especially transient processes that can initiated lower repetition rates, difficult reproduce excitation conditions, or rare samples, encountered high-energy density physics.
    • Relation:
      info:eu-repo/semantics/altIdentifier/pmid/37875533; info:eu-repo/grantAgreement//670787/EU/Planetary diversity: the experimental terapascal perspective/PLANETDIVE; hal-04265682; https://hal.science/hal-04265682; https://hal.science/hal-04265682/document; https://hal.science/hal-04265682/file/s41598-023-44196-2.pdf; PUBMED: 37875533
    • الرقم المعرف:
      10.1038/s41598-023-44196-2
    • الدخول الالكتروني :
      https://hal.science/hal-04265682
      https://hal.science/hal-04265682/document
      https://hal.science/hal-04265682/file/s41598-023-44196-2.pdf
      https://doi.org/10.1038/s41598-023-44196-2
    • Rights:
      info:eu-repo/semantics/OpenAccess
    • الرقم المعرف:
      edsbas.220C4CCA