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Electron correlation and short-range dynamics in attosecond angular streaking

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  • معلومة اضافية
    • بيانات النشر:
      Preprint
    • بيانات النشر:
      American Physical Society (APS), 2020.
    • الموضوع:
      2020
    • نبذة مختصرة :
      We employ the R-matrix with time-dependence method to study attosecond angular streaking of F$^-$. Using this negative ion, free of long-range Coulomb interactions, we elucidate the role of short-range electron correlation effects in an attoclock scheme. Through solution of the multielectron time-dependent Schrodinger equation, we aim to bridge the gap between experiments using multielectron targets, and one-electron theoretical approaches. We observe significant negative offset angles in the photoelectron momentum distributions, despite the short-range nature of the binding potential. We show that the offset angle is sensitive to the atomic structure description of the residual F atom. We also investigate the response of co- and counter-rotating electrons, and observe an angular separation in their emission.
    • File Description:
      application/pdf
    • ISSN:
      2469-9934
      2469-9926
    • الرقم المعرف:
      10.1103/physreva.101.041401
    • الرقم المعرف:
      10.48550/arxiv.2003.12409
    • Rights:
      APS Licenses for Journal Article Re-use
      arXiv Non-Exclusive Distribution
    • الرقم المعرف:
      edsair.doi.dedup.....58c1eb20505e1567aaa05625fed68619