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X-rays induced atomic dynamics in a lithium-borate glass

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  • معلومة اضافية
    • Contributors:
      University of Trento [Trento]; European Synchrotron Radiation Facility (ESRF); Spectroscopies optiques des matériaux verres, amorphes et à nanoparticules (SOPRANO); Institut Lumière Matière [Villeurbanne] (ILM); Université Claude Bernard Lyon 1 (UCBL); Université de Lyon-Université de Lyon-Centre National de la Recherche Scientifique (CNRS)-Université Claude Bernard Lyon 1 (UCBL); Université de Lyon-Université de Lyon-Centre National de la Recherche Scientifique (CNRS); Deutsches Elektronen-Synchrotron [Hamburg] (DESY)
    • بيانات النشر:
      Institute for Condensed Matter Physics, 2019.
    • الموضوع:
      2019
    • نبذة مختصرة :
      The continuous development of synchrotron-based experimental techniques in the X-ray range provides new possibilities to probe the structure and the dynamics of bulk materials down to inter-atomic distances. However, the interaction of intense X-ray beams with matter can also induce changes in the structure and dynamics of materials. A reversible and non-destructive beam induced dynamics has recently been observed in X-ray photon correlation spectroscopy experiments in some oxide glasses at sufficiently low absorbed doses, and is here investigated in a (Li$_2$O)$_{0.5}$(B$_2$O$_3$)$_{0.5}$ glass. The characteristic time of this induced dynamics is inversely proportional to the intensity of the X-ray beam, with a coefficient that depends on the chemical composition and local structure of the probed glass, making it a potentially new tool to investigate fundamental properties of a large class of disordered systems. While the exact mechanisms behind this phenomenon are yet to be elucidated, we report here on the measurement of the exchanged wave-vector (and thus length-scale) dependence of the characteristic time of this induced dynamics, and show that it follows the same power-law observed in vitreous silica. This supports the idea that a unique explanation for this effect in different oxide glasses should be looked for.
      Comment: 9 pages, 4 figures
    • ISSN:
      2224-9079
      1607-324X
    • Rights:
      OPEN
    • الرقم المعرف:
      edsair.doi.dedup.....3277dd682ab17949fba9ae1fe1555554